We probe the electron–phonon coupling for in situ engineered porphyrin-based magnetic molecular layers supported on weakly reactive surfaces. Using high-resolution scanning tunneling microscopy and spectroscopy at 4.5 K we show that the electronic and magnetic properties of the engineered molecules are the result of interplay between many-body spin–flip excitations and electron–phonon interactions.
V. Iancu, K. Schouteden, Z. Li and C. Van Haesendonck, Chem. Commun., 2016, 52, 11359 DOI: 10.1039/C6CC03847F
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