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Issue 40, 2016
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A panchromatic modification of the light absorption spectra of metal–organic frameworks

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Abstract

The optical absorption of UiO-66–NH2 MOF was red-shifted using a diazo-coupling reaction. The modifications performed with naphthols and aniline yielded reddish samples, and the modifications with diphenylaniline yielded dark violet ones. The photocatalytic activity of these modified MOFs was assessed for methylene blue degradation, showing a good performance relative to traditional TiO2. The degradation performance was found to correlate with the red shift of the absorption edge. These findings suggest potential applications of these materials in photocatalysis and in dye sensitized solar cells.

Graphical abstract: A panchromatic modification of the light absorption spectra of metal–organic frameworks

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Supplementary files

Article information


Submitted
16 Mar 2016
Accepted
06 Apr 2016
First published
06 Apr 2016

Chem. Commun., 2016,52, 6665-6668
Article type
Communication

A panchromatic modification of the light absorption spectra of metal–organic frameworks

E. H. Otal, M. L. Kim, M. E. Calvo, L. Karvonen, I. O. Fabregas, C. A. Sierra and J. P. Hinestroza, Chem. Commun., 2016, 52, 6665
DOI: 10.1039/C6CC02319C

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