The local structure of as-synthesised silicalite-1 zeolites is modified using asymmetric R(Pr)3N+ structure directing agents. Using multi-nuclear NMR (1H, 13C, 14N, 19F, 29Si), we show for the first time the ability of these cations to adopt preferential orientations at the zeolite channels’ crossing.
E. Dib, A. Gimenez, T. Mineva and B. Alonso, Dalton Trans., 2015, 44, 16680 DOI: 10.1039/C5DT02558C
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