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Issue 8, 2015
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Competition between electron transfer, trapping, and recombination in CdS nanorod–hydrogenase complexes

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Abstract

Electron transfer from photoexcited CdS nanorods to [FeFe]-hydrogenase is a critical step in photochemical H2 production by CdS–hydrogenase complexes. By accounting for the distributions in the numbers of electron traps and enzymes adsorbed, we determine rate constants and quantum efficiencies for electron transfer from transient absorption measurements.

Graphical abstract: Competition between electron transfer, trapping, and recombination in CdS nanorod–hydrogenase complexes

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Article information


Submitted
21 Dec 2014
Accepted
19 Jan 2015
First published
20 Jan 2015

Phys. Chem. Chem. Phys., 2015,17, 5538-5542
Article type
Communication
Author version available

Competition between electron transfer, trapping, and recombination in CdS nanorod–hydrogenase complexes

J. K. Utterback, M. B. Wilker, K. A. Brown, P. W. King, J. D. Eaves and G. Dukovic, Phys. Chem. Chem. Phys., 2015, 17, 5538
DOI: 10.1039/C4CP05993J

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