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Issue 8, 2015
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Competition between electron transfer, trapping, and recombination in CdS nanorod–hydrogenase complexes

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Abstract

Electron transfer from photoexcited CdS nanorods to [FeFe]-hydrogenase is a critical step in photochemical H2 production by CdS–hydrogenase complexes. By accounting for the distributions in the numbers of electron traps and enzymes adsorbed, we determine rate constants and quantum efficiencies for electron transfer from transient absorption measurements.

Graphical abstract: Competition between electron transfer, trapping, and recombination in CdS nanorod–hydrogenase complexes

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Publication details

The article was received on 21 Dec 2014, accepted on 19 Jan 2015 and first published on 20 Jan 2015


Article type: Communication
DOI: 10.1039/C4CP05993J
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Phys. Chem. Chem. Phys., 2015,17, 5538-5542

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    Competition between electron transfer, trapping, and recombination in CdS nanorod–hydrogenase complexes

    J. K. Utterback, M. B. Wilker, K. A. Brown, P. W. King, J. D. Eaves and G. Dukovic, Phys. Chem. Chem. Phys., 2015, 17, 5538
    DOI: 10.1039/C4CP05993J

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