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Issue 37, 2015
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Electrochemical driven water oxidation by molecular catalysts in situ polymerized on the surface of graphite carbon electrode

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Abstract

A simple strategy to immobilize highly efficient ruthenium based molecular water-oxidation catalysts on the basal-plane pyrolytic graphite electrode (BPG) by polymerization has been demonstrated. The electrode 1@BPG has obtained a high initial turnover frequency (TOF) of 10.47 s−1 at ∼700 mV overpotential, and a high turnover number (TON) up to 31600 in 1 h electrolysis.

Graphical abstract: Electrochemical driven water oxidation by molecular catalysts in situ polymerized on the surface of graphite carbon electrode

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Article information


Submitted
11 Jan 2015
Accepted
19 Mar 2015
First published
20 Mar 2015

Chem. Commun., 2015,51, 7883-7886
Article type
Communication

Electrochemical driven water oxidation by molecular catalysts in situ polymerized on the surface of graphite carbon electrode

L. Wang, K. Fan, Q. Daniel, L. Duan, F. Li, B. Philippe, H. Rensmo, H. Chen, J. Sun and L. Sun, Chem. Commun., 2015, 51, 7883
DOI: 10.1039/C5CC00242G

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