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Issue 14, 2015

Synthesis of nanoporous 1,2,4-oxadiazole networks with high CO2 capture capacity

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Abstract

Developing an adsorbent to mitigate carbon dioxide without large energy penalty is highly desired. Here, we present a silylation synthetic route to form a processable and otherwise impossible porous 1,2,4-oxadiazole network, which achieves 2 mmol g−1 of CO2 capacity owing to a nitrogen-rich structure. This network shows high CO2–N2 selectivity, thermal stability up to 450 °C, and low heat of adsorption (26.4 kJ mol−1), facilitating easy regeneration.

Graphical abstract: Synthesis of nanoporous 1,2,4-oxadiazole networks with high CO2 capture capacity

Supplementary files

Article information


Submitted
31 Oct 2014
Accepted
05 Jan 2015
First published
05 Jan 2015

Chem. Commun., 2015,51, 2915-2917
Article type
Communication

Synthesis of nanoporous 1,2,4-oxadiazole networks with high CO2 capture capacity

D. Ko, H. A. Patel and C. T. Yavuz, Chem. Commun., 2015, 51, 2915 DOI: 10.1039/C4CC08649J

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