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Issue 22, 2014
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Nanocrystalline tin disulfide coating of reduced graphene oxide produced by the peroxostannate deposition route for sodium ion battery anodes

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Abstract

A highly stable sodium ion battery anode was prepared by deposition of hydroperoxostannate on graphene oxide from hydrogen-peroxide-rich solution followed by sulfidization and 300 °C heat treatment. The material was characterized by electron microscopy, powder X-ray diffraction and X-ray photoelectron spectroscopy which showed that the active material is mostly rhombohedral SnS2 whose (001) planes were preferentially oriented in parallel to the graphene oxide sheets. The material exhibited >610 mA h g−1 charge capacity at 50 mA g−1 (with >99.6% charging efficiency) between 0 and 2 V vs. Na/Na+ electrode, high cycling stability for over 150 cycles and very good rate performance, >320 mA h g−1 at 2000 mA g−1.

Graphical abstract: Nanocrystalline tin disulfide coating of reduced graphene oxide produced by the peroxostannate deposition route for sodium ion battery anodes

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Publication details

The article was received on 17 Dec 2013, accepted on 12 Mar 2014 and first published on 29 Apr 2014


Article type: Paper
DOI: 10.1039/C3TA15248K
J. Mater. Chem. A, 2014,2, 8431-8437

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    Nanocrystalline tin disulfide coating of reduced graphene oxide produced by the peroxostannate deposition route for sodium ion battery anodes

    P. V. Prikhodchenko, D. Y. W. Yu, S. K. Batabyal, V. Uvarov, J. Gun, S. Sladkevich, A. A. Mikhaylov, A. G. Medvedev and O. Lev, J. Mater. Chem. A, 2014, 2, 8431
    DOI: 10.1039/C3TA15248K

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