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A facile and eco-friendly approach for the synthesis of mesopore-containing ZSM-5 zeolite with small crystal size was proposed by subtly making use of a coke-deposited spent zeolite catalyst. When used in the methanol to propylene reaction again, the refabricated ZSM-5 catalyst exhibited a much higher propylene selectivity and a longer catalytic lifetime.

Graphical abstract: Facile fabrication of mesopore-containing ZSM-5 zeolite from spent zeolite catalyst for methanol to propylene reaction

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