Issue 4, 2014

Single molecule methods for the study of catalysis: from enzymes to heterogeneous catalysts

Abstract

Structural and temporal inhomogeneities can have a marked influence on the performance of inorganic and biocatalytic systems alike. While these subtle variations are hardly ever accessible through bulk or ensemble averaged activity screening, insights into the molecular mechanisms underlying these diverse phenomena are absolutely critical for the development of optimized or novel catalytic systems and processes. Fortunately, state-of-the-art fluorescence microscopy methods have allowed experimental access to this intriguing world at the nanoscale. In this tutorial review we will first provide a broad overview of key concepts and developments in the application of single molecule fluorescence spectroscopy to (bio)catalysis research. In the second part topics specific to both bio and heterogeneous catalysis will be reviewed in more detail.

Graphical abstract: Single molecule methods for the study of catalysis: from enzymes to heterogeneous catalysts

Article information

Article type
Tutorial Review
Submitted
09 Jul 2013
First published
01 Oct 2013

Chem. Soc. Rev., 2014,43, 990-1006

Single molecule methods for the study of catalysis: from enzymes to heterogeneous catalysts

K. P. F. Janssen, G. De Cremer, R. K. Neely, A. V. Kubarev, J. Van Loon, J. A. Martens, D. E. De Vos, M. B. J. Roeffaers and J. Hofkens, Chem. Soc. Rev., 2014, 43, 990 DOI: 10.1039/C3CS60245A

To request permission to reproduce material from this article, please go to the Copyright Clearance Center request page.

If you are an author contributing to an RSC publication, you do not need to request permission provided correct acknowledgement is given.

If you are the author of this article, you do not need to request permission to reproduce figures and diagrams provided correct acknowledgement is given. If you want to reproduce the whole article in a third-party publication (excluding your thesis/dissertation for which permission is not required) please go to the Copyright Clearance Center request page.

Read more about how to correctly acknowledge RSC content.

Social activity

Spotlight

Advertisements