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Issue 19, 2014
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Combined transparency and optical nonlinearity enhancement in flexible covalent multimers by operating through-space interactions between dipolar chromophores

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Abstract

Subtle manipulation of mutual repulsion and polarisation effects between polar and polarisable chromophores forced in closed proximity allows achieving major (100%) enhancement of the first hyperpolarisability together with increased transparency, breaking the well-known nonlinearity–transparency trade-off paradigm.

Graphical abstract: Combined transparency and optical nonlinearity enhancement in flexible covalent multimers by operating through-space interactions between dipolar chromophores

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Article information


Submitted
18 Feb 2014
Accepted
17 Mar 2014
First published
17 Mar 2014

Phys. Chem. Chem. Phys., 2014,16, 9096-9103
Article type
Paper

Combined transparency and optical nonlinearity enhancement in flexible covalent multimers by operating through-space interactions between dipolar chromophores

V. Parthasarathy, R. Pandey, F. Terenziani, P. K. Das and M. Blanchard-Desce, Phys. Chem. Chem. Phys., 2014, 16, 9096
DOI: 10.1039/C4CP00715H

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