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Issue 64, 2014
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Synthesis of nitrogen heterocycles via α-aminoalkyl radicals generated from α-silyl secondary amines under visible light irradiation

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Abstract

We have succeeded in the visible light-mediated synthetic use of α-aminoalkyl radicals derived from α-silyl secondary amines toward addition to α,β-unsaturated carbonyl compounds. The resulting γ-aminocarbonyl compounds are converted into γ-lactams and pyrroles in a one-pot process.

Graphical abstract: Synthesis of nitrogen heterocycles via α-aminoalkyl radicals generated from α-silyl secondary amines under visible light irradiation

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Supplementary files

Article information


Submitted
23 Apr 2014
Accepted
12 Jun 2014
First published
16 Jun 2014

This article is Open Access

Chem. Commun., 2014,50, 8900-8903
Article type
Communication
Author version available

Synthesis of nitrogen heterocycles via α-aminoalkyl radicals generated from α-silyl secondary amines under visible light irradiation

K. Nakajima, M. Kitagawa, Y. Ashida, Y. Miyake and Y. Nishibayashi, Chem. Commun., 2014, 50, 8900
DOI: 10.1039/C4CC03000A

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