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Issue 52, 2017
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Tracking thermal-induced amorphization of a zeolitic imidazolate framework via synchrotron in situ far-infrared spectroscopy

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Abstract

We present the first use of in situ far-infrared spectroscopy to analyze the thermal amorphization of a zeolitic imidazolate framework material. We explain the nature of vibrational motion changes during the amorphization process and reveal new insights into the effect that temperature has on the Zn–N tetrahedra.

Graphical abstract: Tracking thermal-induced amorphization of a zeolitic imidazolate framework via synchrotron in situ far-infrared spectroscopy

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Article information


Submitted
15 Mar 2017
Accepted
06 Jun 2017
First published
06 Jun 2017

Chem. Commun., 2017,53, 7041-7044
Article type
Communication

Tracking thermal-induced amorphization of a zeolitic imidazolate framework via synchrotron in situ far-infrared spectroscopy

M. R. Ryder, T. D. Bennett, C. S. Kelley, M. D. Frogley, G. Cinque and J. Tan, Chem. Commun., 2017, 53, 7041
DOI: 10.1039/C7CC01985H

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