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We report a fast, scalable, and low energy approach to synthesize battery-grade Li4Ti5O12 (LTO). Low-temperature, microwave-assisted solvothermal synthesis yields nanoplatelets that self-assemble into microspheres. Following calcination, these microspheres exhibit capacities of 170 mAh g−1 and a capacity retention of 99% over 100 cycles.

Graphical abstract: Rapid, microwave-assisted synthesis of battery-grade lithium titanate (LTO)

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