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Issue 21, 2013

Strong-pump strong-probe spectroscopy: effects of higher excited electronic states

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Abstract

The present paper is devoted to the simulation of (integral and dispersed) pump–probe signals in the nonperturbative regime for a series of material systems with multiple electronic states and excited-state absorption. We show that strong-pump strong-probe spectroscopy permits the probing of vibrational wavepackets in high-lying and/or short-lived excited electronic states with a time resolution which is not limited by the pulse durations. The field strength can be regarded as an additional experimentally controllable parameter, which can be tuned to maximize the spectroscopic information for a given material system.

Graphical abstract: Strong-pump strong-probe spectroscopy: effects of higher excited electronic states

Article information


Submitted
11 Dec 2012
Accepted
21 Mar 2013
First published
22 Mar 2013

Phys. Chem. Chem. Phys., 2013,15, 8119-8131
Article type
Paper

Strong-pump strong-probe spectroscopy: effects of higher excited electronic states

M. F. Gelin, D. Egorova and W. Domcke, Phys. Chem. Chem. Phys., 2013, 15, 8119 DOI: 10.1039/C3CP44454F

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