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Issue 81, 2013
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Non-enzymatic acylative kinetic resolution of primary allylic amines

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Abstract

A non-enzymatic acetyl transfer-based kinetic resolution of primary allylic amines is reported. The process involves the use of (1S,2S)-1 in conjunction with a supported ammonium salt and affords the corresponding enantio-enriched N-acetylated allylic amines with unprecedented levels of selectivity (s-factors up to 34).

Graphical abstract: Non-enzymatic acylative kinetic resolution of primary allylic amines

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Article information


Submitted
18 Jul 2013
Accepted
13 Aug 2013
First published
14 Aug 2013

Chem. Commun., 2013,49, 9338-9340
Article type
Communication

Non-enzymatic acylative kinetic resolution of primary allylic amines

A. Kolleth, M. Cattoen, S. Arseniyadis and J. Cossy, Chem. Commun., 2013, 49, 9338
DOI: 10.1039/C3CC45453C

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