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Abstract | Cited by

Malonganenone B (1) exhibits an unusual H–D exchange of a formyl proton when in deuteric-NMR solvents. Synthetic and kinetic investigations were made to probe the mechanism of this exchange, which appears to occur via an uncommon and transient amine–amide NHC intermediate.

Graphical abstract: Studies of the H–D exchange mechanism of malonganenone B

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