Issue 10, 2012
From the journal:

Energy & Environmental Science

Towards the development of a hydrogen battery

Albert Boddien,a   Christopher Federsel,a   Peter Sponholz,a   Dörthe Mellmann,a   Ralf Jackstell,a   Henrik Junge,a   Gabor Laurenczy*b  and  Matthias Beller*a  

* Corresponding authors

a Leibniz-Institut für Katalyse e.V. an der Universität Rostock, Albert-Einstein Strasse 29a, 18059 Rostock, Germany
E-mail: matthias.beller@catalysis.de
Fax: +49 381-1281-5000

b Institut des Sciences et Ingénierie Chimiques, École Polytechnique Fédérale de Lausanne (EPFL), 1015 Lausanne, Switzerland
E-mail: gabor.laurenczy@epfl.ch
Fax: +41 21-693-9780

Abstract

A novel Ru-catalyzed hydrogenation of carbon dioxide proceeds with an unprecedented high formic acid to amine ratio (AAR of 2.69), which results in an improved energy content. The presented catalyst system allows for reversible fast hydrogen loading (even at RT) and unprecedented unloading (TON for H2 liberation of 800 000).

Graphical abstract: Towards the development of a hydrogen battery

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Article information

DOI
https://doi.org/10.1039/C2EE22043A
Article type
Communication
Submitted
25 Apr 2012
Accepted
11 Jul 2012
First published
12 Jul 2012

Energy Environ. Sci., 2012,5, 8907-8911

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Towards the development of a hydrogen battery

A. Boddien, C. Federsel, P. Sponholz, D. Mellmann, R. Jackstell, H. Junge, G. Laurenczy and M. Beller, Energy Environ. Sci., 2012, 5, 8907 DOI: 10.1039/C2EE22043A

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