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Issue 22, 2012
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Polyoxometalate water oxidation catalysts and the production of green fuel†

Hongjin Lv,a   Yurii V. Geletii,a   Chongchao Zhao,a   James W. Vickers,a   Guibo Zhu,a   Zhen Luo,a   Jie Song,a   Tianquan Lian,a   Djamaladdin G. Musaevb  and  Craig L. Hill*a  
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* Corresponding authors

a Department of Chemistry, Emory University, Atlanta, GA, USA
E-mail: chill@emory.edu
Fax: +1 404-727-6076
Tel: +1 404-727-6611

b Cherry L. Emerson Center for Scientific Computation, Emory University, Atlanta, GA, USA

Abstract

In the last five years and currently, research on solar fuels has been intense and no sub-area in this field has been more active than the development of water oxidation catalysts (WOCs). In this timeframe, a new class of molecular water oxidation catalysts based on polyoxometalates have been reported that combine the advantages of homogeneous and heterogeneous catalysts. This review addresses central issues in green energy generation, the challenges in water oxidation catalyst development, and the possible uses of polyoxometalates in green energy science.

Graphical abstract: Polyoxometalate water oxidation catalysts and the production of green fuel

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Article information

https://doi.org/10.1039/C2CS35292C
Submitted
30 Jul 2012
First published
12 Sep 2012
Chem. Soc. Rev., 2012,41, 7572-7589
Article type
Critical Review
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Polyoxometalate water oxidation catalysts and the production of green fuel

H. Lv, Y. V. Geletii, C. Zhao, J. W. Vickers, G. Zhu, Z. Luo, J. Song, T. Lian, D. G. Musaev and C. L. Hill, Chem. Soc. Rev., 2012, 41, 7572
DOI: 10.1039/C2CS35292C

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