Oxidative imination of toluenes catalyzed by Pd–Au/silica gel under mild reaction conditions

Xinjiang Cui; Feng Shi; Youquan Deng

doi:10.1039/C2CC31438J

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Oxidative imination of toluenes catalyzed by Pd–Au/silica gel under mild reaction conditions†

Xinjiang Cui,^ab Feng Shi*^a and Youquan Deng^a

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* Corresponding authors

^a Centre for Green Chemistry and Catalysis, Lanzhou Institute of Chemical Physics, CAS Middle Tian Road, 18, Lanzhou, China
E-mail: fshi@licp.cas.cn
Fax: (+86)-931-8277088

^b Graduate School of the Chinese Academy of Sciences, Beijing, China

Abstract

A Pd–Au/SiO₂ catalyst was prepared for the oxidative imination of toluenes with up to 99% yields in the absence of dehydrating agents under mild conditions. Nanoparticles with a PdO layer and PdO–Au core may be the active structure for the reaction.

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Article information

DOI: https://doi.org/10.1039/C2CC31438J
Article type: Communication
Submitted: 27 Feb 2012
Accepted: 08 Jun 2012
First published: 11 Jun 2012

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Chem. Commun., 2012,48, 7586-7588

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Oxidative imination of toluenes catalyzed by Pd–Au/silica gel under mild reaction conditions

X. Cui, F. Shi and Y. Deng, Chem. Commun., 2012, 48, 7586 DOI: 10.1039/C2CC31438J

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Chemical Communications

Oxidative imination of toluenes catalyzed by Pd–Au/silica gel under mild reaction conditions†

Abstract

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Oxidative imination of toluenes catalyzed by Pd–Au/silica gel under mild reaction conditions

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