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Abstract | Cited by

Two different strategies for the synthesis of functionalised γ-lactones from δ-lactones are described and used in a convergent synthesis of (+)-mupirocin H. The total synthesis is versatile and may be readily adapted for the preparation of further truncated metabolites from Pseudomonas fluorescens.

Graphical abstract: γ-lactones from δ-lactones: total synthesis of the biosynthetic derailment product mupirocin H

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