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Issue 28, 2011
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Tunable single-site ruthenium catalysts for efficient water oxidation

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Abstract

The catalyticwater oxidation activity of mononuclear ruthenium complexes comprising a pyridine-functionalized abnormal triazolylidene ligand can be adjusted by modification of the triazolylidene substituents, which is readily achieved through click-type cycloaddition chemistry, affording some of the most active ruthenium catalysts known thus far for water oxidation (TONs > 400, TOFs close to 7000 h−1).

Graphical abstract: Tunable single-site ruthenium catalysts for efficient water oxidation

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Article information


Submitted
04 May 2011
Accepted
01 Jun 2011
First published
16 Jun 2011

Chem. Commun., 2011,47, 8058-8060
Article type
Communication

Tunable single-site ruthenium catalysts for efficient water oxidation

L. Bernet, R. Lalrempuia, W. Ghattas, H. Mueller-Bunz, L. Vigara, A. Llobet and M. Albrecht, Chem. Commun., 2011, 47, 8058
DOI: 10.1039/C1CC12615F

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