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Issue 11, 2011
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Functionalisation of aldehydesvia aerobic hydroacylation of azodicarboxylates ‘on’ water

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Abstract

Herein we report the functionalisation of aldehydesvia hydroacylation of azodicarboxylates. A range of functionalised aldehydes are employed as the limiting reagent including chiral non-racemic aldehydes bearing α-stereocentres which are functionalised giving access to enantiomerically pure products. The resultant hydrazides can be employed as acyl donors in the synthesis of amides.

Graphical abstract: Functionalisation of aldehydesvia aerobic hydroacylation of azodicarboxylates ‘on’ water

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Article information


Submitted
20 Oct 2010
Accepted
21 Dec 2010
First published
01 Feb 2011

Chem. Commun., 2011,47, 3269-3271
Article type
Communication

Functionalisation of aldehydesvia aerobic hydroacylation of azodicarboxylates ‘on’ water

V. Chudasama, J. M. Ahern, D. V. Dhokia, R. J. Fitzmaurice and S. Caddick, Chem. Commun., 2011, 47, 3269
DOI: 10.1039/C0CC04520A

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