Jump to main content
Jump to site search

Issue 48, 2010
Previous Article Next Article

Local control of multidimensional dynamics

Author affiliations

Abstract

The control of chemical reactions has been a target for researchers since the development of lasers which operated on a timescale fast enough to follow nuclear motion. Since then a number of schemes have been developed, each proving successful in a selection of systems. In this paper we present results obtained following the implementation of local control theory together with the multi-configuration time dependent Hartree quantum dynamics algorithm, aiming to efficiently design control pulses for polyatomic systems. Control of multidimensional models of cyclobutadiene and pyrazine are presented and discussed. These results represent a starting point for further studies, showing the distinct advantages of using this approach for controlling chemical reactions.

Graphical abstract: Local control of multidimensional dynamics

Back to tab navigation

Article information


Submitted
02 Mar 2010
Accepted
05 May 2010
First published
23 Jun 2010

Phys. Chem. Chem. Phys., 2010,12, 15616-15627
Article type
Paper

Local control of multidimensional dynamics

T. J. Penfold, G. A. Worth and C. Meier, Phys. Chem. Chem. Phys., 2010, 12, 15616
DOI: 10.1039/C003768K

Social activity

Search articles by author

Spotlight

Advertisements