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Although the adsorption of benzenethiols (BT) on Au(111) usually leads to the formation of disordered phases, we demonstrate here that the displacement of preadsorbed cyclohexanethiol self-assembled monolayers (SAMs) on Au(111) by BT molecules can be a successful approach to obtain two-dimensional BT SAMs with long-range ordered domains.

Graphical abstract: Two-dimensional ordering of benzenethiol self-assembled monolayers guided by displacement of cyclohexanethiols on Au(111)

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