Laser control of physicochemical processes; experiments and applications†
Abstract
This review outlines experimental advances that have been made in laser control of physicochemical processes, with an emphasis on the 2004–2006 period. After a brief introduction, an overview of the technology available for delivering ultrashort shaped femtosecond pulses is presented. Special attention is given to recent progress on laser control of chemical reactions and the application of this concept to molecular identification. We also cover control of simpler systems such as atoms and diatomic molecules. Laser control of large molecules in solution is also reviewed from the point of view of selective spectroscopic excitation with applications in