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Abstract | Cited by

The complexes [Ru(CN)4(HAT)]2−, [{Ru(CN)4}2(μ2-HAT)]4− and [{Ru(CN)4}3(μ3-HAT)]6− (HAT = hexaaza-triphenylene) contain four, eight and twelve externally-directed cyanide ligands, respectively; they show strongly solvatochromic and intense MLCT absorptions, and [3]6− forms a high-dimensionality cyanide-bridged coordination network with Nd(III), in which Ru → Nd energy transfer results in sensitised near-IR luminescence.

Graphical abstract: Polynuclear cyanoruthenate chromophores based on hexaaza-triphenylene containing up to twelve cyanides: photophysical and structural properties

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