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Mild catalytic dehydrogenation of cycloalkanes (cyclo-C5H10, cyclo-C6H12, cyclo-C8H16) and aziridination of resulting olefins is reported with PhINTs and copper-[2.1.1]-(2,6)-pyridinophane (L) complexes LCuXn (n = 1, 2; X = Cl, OTf) “activated” with NaBArF4 in dichloromethane solution.

Graphical abstract: Facile alkane functionalization in copper-[2.1.1]-(2,6)-pyridinophane-PhINTs systems

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