The crystalline nitroxide biradical, 1,2,5,7-tetramethyl-2,6-diazaadamantane N,N′-dioxyl, shows ferromagnetic interactions in the solid: a positive Weiss-constant θ= 10 K, a large χT increase at low temperature (T < 20 K) and a magnetisation curve consistent with a total spin S= 6.
R. Chiarelli, A. Rassat and P. Rey, J. Chem. Soc., Chem. Commun., 1992, 1081 DOI: 10.1039/C39920001081
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