At a CH4/O2 ratio of ca. 3 the LiNiO2 and NaMnO4/MgO catalysts generate gas phase methyl radicals as effectively as a Li+/MgO catalyst, which indicates that the mechanism for ethane formation over all three catalysts is the same and involves the coupling of these gas phase radicals.
Y. Tong and J. H. Lunsford, J. Chem. Soc., Chem. Commun., 1990, 792 DOI: 10.1039/C39900000792
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