Reduction of copper(II) in the presence of cyanoguanidine {cnge; (NH2)2CNCN} affords the dimeric cation, [Cu2(cnge)4]2+, which contains trigonal planar copper(I) centres and which stacks such that each copper(I) centre may interact with the π-system of the nitrile function of an adjacent cnge molecule.
M. J. Begley, P. Hubberstey and P. H. Walton, J. Chem. Soc., Chem. Commun., 1989, 502 DOI: 10.1039/C39890000502
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