The He(I) photoelectron (PE) spectra of 1,8-diazabiphenylene (1) and 2,7-diazabiphenylene (2) have been investigated. To aid the interpretation of the PE spectra semiempirical MO calculations have been performed. The ionization transitions from the lone-pair orbitals have been assigned to be ca. 9.6 and 9.7 eV for (1) and (2), respectively.
H. Yamaguchi, M. Higashi, J. A. H. MacBride and R. Gleiter, J. Chem. Soc., Faraday Trans. 2, 1985, 81, 1831 DOI: 10.1039/F29858101831
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