During flow pyrolysis experiments involving sulphur dicyanide vapour, S(CN)2, a new microwave spectrum was detected, analysis of which indicates that S(CN)2 isomerises to cyanogen isothiocyanate, NCNCS, at 850 °C.
M. A. King and H. W. Kroto, J. Chem. Soc., Chem. Commun., 1980, 606a DOI: 10.1039/C3980000606A
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