The structure of the crystalline addition product of dinitrogen trioxide to 2-methylpropene is established unequivocally as trans-2-methyl-2-nitroso-1-nitropropane dimer indicating that the addition proceeds at least partially if not predominantly by a radical mechanism.
J. Pfab, J. Chem. Soc., Chem. Commun., 1977, 766 DOI: 10.1039/C39770000766
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