The correlation of the spectra of the title compounds with those of the free donors is consistent with simple σ donor–acceptor bonding in NH3BH3, but with σ-donation and π-back-donation in BH3CO; recent calculations agree well with experiment for NH3BH3 but less well for BH3CO.
D. R. Lloyd and N. Lynaugh, J. Chem. Soc. D, 1970, 1545 DOI: 10.1039/C29700001545
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