Hybrid magneto-excitonic polariton metastructures: room-temperature strong coupling in all-oxide platforms

Abstract

Breaking optical reciprocity at room temperature in a fully dielectric platform remains a demanding yet impactful goal for integrated photonics. In this work we design and numerically demonstrate a lithography-defined, all-oxide metastructure that merges ferrimagnetic CoFe2O4 nanodisks with Mn-doped ZnO (ZnO:Mn) nanodisks, separated by a sub-2 nm Al2O3 spacer. This geometry, refined through detailed parameter sweeps and alignment tolerances captured in our original design notes, supports hybrid magneto-exciton polaritons with Rabi splittings up to 120 meV and cooperativity factors exceeding 5 at 300 K—without cryogenics or metallic losses. Finite-difference time-domain and micromagnetic simulations, combined with coupled-mode modelling, reveal broadband (>20 nm) bias-tunable nonreciprocal transmission windows whose spectral positions can be engineered via geometry, Mn content, and interlayer spacing. Our findings validate the concept sketched in the initial design drafts: an oxide-exclusive, CMOS-compatible platform delivering bias-reconfigurable spin–photon coupling, scalable fabrication, and chemical-thermal stability. The approach bridges fundamental magneto-optical physics with practical on-chip implementations, offering a clear pathway toward energy-efficient isolators, routers, and phase-controlled photonic components operating at ambient conditions.

Graphical abstract: Hybrid magneto-excitonic polariton metastructures: room-temperature strong coupling in all-oxide platforms

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Article information

Article type
Paper
Submitted
22 Aug 2025
Accepted
13 Nov 2025
First published
14 Nov 2025

J. Mater. Chem. C, 2026, Advance Article

Hybrid magneto-excitonic polariton metastructures: room-temperature strong coupling in all-oxide platforms

A. Vaghef-Koodehi, M. Nikoufard and Y. Bahari, J. Mater. Chem. C, 2026, Advance Article , DOI: 10.1039/D5TC03175C

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