Open Access Article
Kumpei Shiraishi
*a and
Hideyuki Mizuno
b
aSANKEN, University of Osaka, 8-1 Mihogaoka, Ibaraki, Osaka 567-0047, Japan. E-mail: kumpei.shiraishi@sanken.osaka-u.ac.jp
bGraduate School of Arts and Sciences, University of Tokyo, 3-8-1 Komaba, Meguro, Tokyo 153-8902, Japan
First published on 10th February 2026
We investigate sample-to-sample fluctuations of the shear modulus in ensembles of particle packings near the jamming transition. Unlike the average modulus, which exhibits distinct scaling behaviours depending on the interparticle potential, the fluctuations obey a critical exponent that is independent of the potential. Furthermore, this scaling behaviour has been confirmed in two-dimensional packings, indicating that it holds regardless of spatial dimension. Using this scaling law, we discuss the relationship predicted by heterogeneous-elasticity theory between elastic-modulus fluctuations and the Rayleigh scattering of sound waves across different pressures. Our numerical results provide a useful foundation for developing a unified theoretical description of the jamming critical phenomenon.
One of the central challenges in statistical physics is the understanding of phase transitions and critical phenomena.16–19 In this context, theoretical tools such as mean-field theory and, more importantly, the renormalization group have been developed, and it has become clear that fluctuations play a crucial role in critical behaviour. In particular, as a system approaches a critical point, both the fluctuations and the associated correlation length scales diverge, leading to various anomalies at the critical point. In the field of jamming transition, some works have followed this line of research, including scaling collapse and finite-size scaling,9,20,21 diverging length scales,3,10,22,23 and Widom scaling hypothesis.24 Thus, understanding how fluctuations in physical quantities behave near the jamming critical point remains an important issue. Despite its relevance, the study of fluctuations in jamming systems is still limited, and further development is anticipated.25–28
Beyond their relevance in statistical physics, fluctuations in elastic moduli play an essential role in the theoretical description of the anomalous properties of amorphous solids. Among the various theoretical frameworks,29–34 the heterogeneous-elasticity theory (HET)35–39 is one of the most well-established approaches for describing the anomalous behaviour of amorphous materials such as jammed solids. HET postulates that the local shear modulus exhibits spatial fluctuations throughout the system, and extensive numerical studies have indeed confirmed the existence of such elastic heterogeneity in amorphous systems.40–42 Within this theoretical framework, the so-called disorder parameter γ, which quantifies the variance of local shear moduli, acts as a key control parameter.36 In the standard formulation of HET, the distribution of local shear moduli is assumed to be Gaussian, and its mean value and standard deviation serve as inputs for computing macroscopic observables. This formulation successfully accounts for a variety of universal features of amorphous solids. For example, the low-frequency vibrational modes in excess over the Debye prediction (the boson peak) can be captured within HET, with both their characteristic frequency and intensity expressed as functions of γ. Likewise, the theory predicts a Rayleigh-type frequency dependence of the acoustic attenuation, Γ∼Ωd+1 (Γ is the attenuation coefficient and Ω is the propagation frequency), which is also observed in experiments on glasses.43,44 The prefactor of this relation, corresponding to the strength of Rayleigh scattering, is again determined by γ, linking vibrational and transport anomalies to the underlying elastic heterogeneity. These theoretical predictions, spanning both vibrational spectra14,45,46 and acoustic attenuation,14,47,48 have been extensively tested through numerical simulations.
Another major theoretical framework developed to describe and predict the properties of amorphous solids is the effective medium theory (EMT), which is based on spring-network models.49 While HET treats the spatial fluctuations of local shear moduli as the sole mesoscale input, EMT instead relies on microscopic parameters, namely the mean coordination number z and the contact strain e, often referred to as the pre-stress. Despite this difference in the scale of description, EMT successfully reproduces the same key features of vibrational and scattering phenomena as HET, including the emergence of the boson peak and the Rayleigh-type acoustic attenuation. Given that both theories capture similar physical phenomena from different levels of description, it is natural to expect that they are connected via an appropriate coarse-graining procedure. However, the precise nature of this connection remains elusive. One major reason for this persistent gap is the limited numerical characterisation of fluctuations of elastic modulus. From this perspective, a detailed characterisation of local shear modulus fluctuations is of particular theoretical significance, particularly for bridging the gap between these two frameworks.
In this work, we characterise the sample-to-sample fluctuations of elastic moduli in ensembles of jammed packings by means of numerical simulation. These fluctuations are believed to encode information equivalent to the disorder parameter in HET.50,51 We focus on two prototypical models of jammed amorphous solids: harmonic spheres and Hertzian spheres. Our results reveal that, while the average elastic modulus exhibits a model-dependent scaling behaviour, its fluctuations diverge in a manner independent of the interaction potential. This critical scaling is also observed in two-dimensional packings. Finally, we discuss the theoretical implications of these findings, with particular emphasis on their relevance to the HET prediction on acoustic attenuation in amorphous solids.
![]() | (1) |
:
50 binary mixtures of particles whose diameters are σ and 1.4σ with identical mass m. The number of particles in the system is denoted as N. Masses, lengths, and energies are measured in units of m, σ, and ε, respectively. The number density is expressed as ρ = N/Ld, where d = 3 is the spatial dimension.
is reached. Then, we perform the global compression/decompression to generate packings at a given target pressure p.53 For harmonic spheres, pressures range over p = 10−2, 10−3, …, 10−6 for all system sizes. For Hertzian spheres, the highest pressure is p = 10−2 for all system sizes, and the lowest pressure is p = 10−8 for N = 2000. For the case of N = 32
000, the lowest pressure is p = 10−7. A packing ensemble prepared with the compression/decompression-only protocols may contain samples that have finite pressure but are unstable to shear.54 We discard such samples with a negative shear modulus when constructing the ensembles. The sizes of ensembles used in this study are given in Appendix A. After packings are generated, we recursively remove rattler particles whose number of contacts Nc satisfies Nc ≤ d.55
The elastic modulus is decomposed into two components, the affine and non-affine modulus: G = GA − GN.59,60 The affine modulus (Born–Huang term) is the second derivative of total potential energy E, defined as
![]() | (2) |
![]() | (3) |
The second term GN is due to non-affine relaxation. This term is evaluated with the Hessian matrix56–58
![]() | (4) |
![]() | (5) |
−1·Ξ.56–59,66 This displacement field δu (3N-dimensional vector) is usually obtained though the decomposition of Ξ with the normal modes of
.56–58 However, this method is computationally hard when the size of matrix becomes large. Therefore, we obtain the non-affine displacements δu via the FIRE minimisation of a cost function
![]() | (7) |
. This iterative method yields displacements that are identical to the direct solution of the linear equation
·δu = Ξ within numerical tolerance.
In the harmonic limit, the energy change ΔE caused by relative displacements {ui} from the mechanically equilibrated position {ri} takes the form3,4,9,61,68
![]() | (8) |
·u. Because the contact force fij = −v′(rij) is always repulsive in the jammed packings, the original state is called the stressed system. On the other hand, we have also studied the shear modulus of the unstressed system,4 where we remove fij in the Hessian matrix while maintaining kij. This case corresponds to the system where we replace the interactions between particles with relaxed (unstretched) springs of each stiffness kij. In practice, we omit the first derivatives in the Hessian matrix in the cost function (7) when calculating the shear modulus of the unstressed system. We denote the shear modulus of the stressed system by G1 and that of the unstressed system by G0.
| G ∼ p(α−3/2)/(α−1). | (9) |
In addition, the excess contact number δz = z − ziso, which quantifies the distance from the isostatic point at the onset of jamming,4,6 is known to scale as6:
| δz ∼ p1/(2α−2). | (10) |
Here, ziso = 2d(1 − 1/N) is the isostatic contact number that satisfies the Maxwell criterion, and the 1/N correction arises from the global zero-frequency translational modes of the finite-size systems.20 Combining the two scaling relations yields G ∼ δz for harmonic spheres (α = 2), and G ∼ δz2 for Hertzian spheres (α = 5/2). As clearly shown in Fig. 1, our numerical data are consistent with these predictions: harmonic spheres exhibit the scaling 〈G1〉 ∼ δz, while Hertzian spheres obey 〈G1〉 ∼ δz2, where 〈·〉 denotes the ensemble average.
![]() | ||
| Fig. 1 Critical scaling of the average shear moduli 〈G1〉 and 〈G0〉/2 for harmonic and Hertzian packings with N= 32000. The solid and dashed lines represent 〈G〉 ∼ δz and 〈G〉 ∼ δz2, respectively. | ||
We now turn to the unstressed modulus G0. Similar to the stressed modulus G1, the unstressed modulus G0 follows the same scaling laws for harmonic and Hertzian spheres, as shown in Fig. 1. In addition, according to the EMT for spring networks, the stressed shear modulus G1 is expected to be twice the unstressed modulus G0 near the jamming point.49 To test this prediction, we plot G0/2 for both types of packings in Fig. 1. Near the jamming transition, 〈G0〉/2 collapses onto 〈G1〉, indicating good quantitative agreement with EMT. However, further from the transition, 〈G1〉 exceeds 〈G0〉/2, suggesting that the pre-stress e at higher pressure deviates from its critical value ec.49 Overall, Fig. 1 clearly demonstrates that both 〈G0〉 and 〈G1〉 obey the same scaling law within each model, while the scaling exponent itself depends on the interaction potential.
z) computed from the ensemble of Hertzian packings with N = 32
000. To facilitate comparison across different pressures, we rescale the variable as
z = δz/〈δz〉 − 1. As illustrated in Fig. 2(a), the distribution is symmetric and approximately Gaussian in shape. As the pressure decreases and the system approaches the jamming transition, the distribution broadens.
We next quantify the pressure dependence of these fluctuations across the ensemble. To do so, we adopt a disorder quantifier for a generic observable X, defined as28
![]() | (11) |
Fig. 3 displays χδz for both interaction types across various system sizes. Harmonic spheres exhibit scaling behaviour χδz ∼ δz−2/5, consistent with the findings of Giannini and coworkers,28 albeit subject to finite-size effects. On the other hand, contact-number fluctuations χδz of the Hertzian spheres follow a similar scaling behaviour with δz. Giannini and coworkers identified distinct regimes within the jammed phase based on the behaviour of χδz. They reported that χδz becomes independent of system size at high pressures, where the scaling becomes steeper, with a more negative exponent. According to their analysis, this crossover occurs at δz ≈ 7 × 10−1, and they referred to the corresponding high-δz region as the glassy regime (δz ≳ 7 × 10−1). Our results for both harmonic and Hertzian spheres are consistent with these observations, although we do not explore this aspect in further detail here.
![]() | ||
| Fig. 3 Critical fluctuations of the excess contact number δz. The dashed line represents the scaling χδz ∼ δz−2/5. The shaded region marks the glassy regime, δz ≳ 7 × 10−1, where this scaling behaviour is no longer expected to hold.28 | ||
Compared with the excess contact number δz (Fig. 2(a)), both moduli exhibit broader distributions at the same system size. As the pressure is lowered and the system approaches the jamming transition, these distributions become broader, mirroring the trend observed in P(δz). The distinction between G1 and G0 is also evident in Fig. 2(b). At a given pressure, G0 displays a narrower distribution than G1. Although both distributions broaden as pressure decreases, G0 consistently remains narrower than G1, yet both are wider than the distribution of δz.
The shapes of the distributions also differ notably. At high pressure (p = 10−2), both G0 and G1 exhibit symmetric distributions. However, at lower pressures (e.g., p = 10−4), the peak of P(Ĝ1) shifts towards positive values (Ĝ1 > 0), and the distribution becomes skewed. This asymmetry becomes more pronounced as the system approaches the jamming point (p = 10−6). By contrast, P(Ĝ0) retains a symmetric, Gaussian-like shape throughout this pressure range.
Such non-Gaussian behaviour in the distribution of G1 has been previously reported,50 and the skewness is attributed to spatially localised vibrational modes at low frequencies, which are suppressed in the unstressed system.11 Moreover, outliers are found only in the distribution of the stressed modulus. To quantify this, we examine the minimum and maximum values of Ĝ0 and Ĝ1 within the ensemble. While these rare samples are not visible in Fig. 2(b) due to limited statistics, we observe that |minĜ1|/maxĜ1 ≈ 2.5 to 4, indicating the presence of samples with anomalously small G1. Consequently, a Shapiro–Wilk test applied to the raw data returns p-values close to zero, confirming strong deviation from normality. In contrast, for the unstressed modulus G0, we find |minĜ0|/maxĜ0 ≈ 1, indicating an absence of outliers. The Shapiro–Wilk test on G0 returns p-values of approximately 0.8 or larger, even without removing any outlier data, suggesting consistency with a Gaussian distribution.
We now quantify the sample-to-sample fluctuations in the shear moduli. As noted above, the distribution of G1 is markedly different from Gaussian and includes significant outliers, making the standard definition of the fluctuation χG problematic. To address this, a more robust, median-based measure has been proposed:71
![]() | (12) |
Fig. 4 shows the fluctuation of the shear modulus as a function of δz for both moduli. For the unstressed modulus G0, the fluctuations exhibit a clear scaling relation: χG ∼ δz−1/2. Finite-size effects appear negligible in this case, consistent with the narrower distribution of G0 compared to G1 (Fig. 2(b)). For the stressed modulus G1, the fluctuations approach the same scaling χG ∼ δz−1/2 as the system size increases. At higher pressures (i.e., larger δz), the scaling breaks down, consistent with the identification of the glassy regime at δz ≳ 7 × 10−1 by Giannini and coworkers.28 An important conclusion from Fig. 4 is that, in contrast with the average shear modulus (Fig. 1), the fluctuation χG appears independent of the interaction potential exponent α. For harmonic spheres, the scaling exponent is in agreement with previous findings.21,28
![]() | ||
| Fig. 4 Critical fluctuations of the shear moduli. The unstressed modulus G0 and stressed modulus G1 are shown in panels (a) and (b), respectively. The dashed lines indicate the scaling χG ∼ δz−1/2. The legend is identical to that in Fig. 3. The shaded region denotes the glassy regime.28 | ||
As stated in the Introduction, the divergence of fluctuations implies the divergence of associated correlation lengths. Our results indicate that the exponent governing the length scale associated with contact-number fluctuations depends on spatial dimension, whereas the length scale associated with elastic-modulus fluctuations exhibits the same scaling behaviour in both two and three dimensions. The exponent controlling the divergence of elastic-modulus fluctuations coincides with that of the correlation length lc ∼ δz−1/2, which characterises low-frequency vibrational modes and diverges at the jamming transition.10 Crucially, the shear modulus of jammed packing is significantly influenced by non-affine responses to the deformation, which are known to be spatially organised over lc under global shear.72 Just as the four-point susceptibility reflects the growth of domain size of dynamic heterogeneity in glass-forming liquids, the divergence of χG manifests the increasing correlation length of the non-affine displacement fields. As the system approaches the jamming transition, these displacements become increasingly correlated over larger distances, leading to greater variability in the shear modulus between different samples. This length scale lc related to elastic-modulus fluctuations also manifests itself in vibrational modes10,23,73 and responses to local perturbation,22 and these behaviours can also be captured within EMT.49,74 The fact that χG ∼ δz−1/2 ∼ lc holds across different interaction potentials and spatial dimensions strongly suggests that the elastic criticality is robustly controlled by this mesoscopic length scale, regardless of local microscopic details. By contrast, the physical implication of the length scale associated with contact-number fluctuations remains unclear. However, our results highlight the fact that those fluctuations obey different scaling exponents in two and three dimensions, while the average contact number follows a single exponent. This suggests that the spatial correlation of the contact network or geometric constraints may involve different characteristic features in dimensions.
Finally, we situate our results on elastic fluctuations in the context of the HET, which provides a theoretical framework for describing sound attenuation in amorphous solids. According to HET, the attenuation coefficient Γ and the propagation frequency Ω are related through the Rayleigh scaling35
![]() | (13) |
and a0 = ρ−1/d is the characteristic interparticle spacing. It should be noted that HET does not provide a fully quantitative prediction of the absolute magnitude of Γ, and a system-dependent rescaling factor is generally required to achieve quantitative agreement with numerical data.50,77
Detailed numerical simulations have elucidated the jamming scaling laws governing sound attenuation.14 In the low-frequency regime of the Rayleigh scattering, it follows
![]() | (14) |
Recent simulations of soft-core and Lennard-Jones systems have demonstrated that this disorder parameter could be estimated from sample-to-sample fluctuations50,51,78 by assuming the spatial correlations of local elastic moduli are short-ranged and saturate upon coarse-graining.40,41,61,79 This approach also has the merit of sidestepping the direct evaluation of local elastic moduli,41,47 and it is claimed that spatial fluctuations of shear modulus γ can be replaced by the sample-to-sample fluctuations χG2.50,51 Our present result of jammed packings shows that χG2 ∼ δz−1 regardless of the spatial dimension, and this is indeed aligned with numerical simulations of acoustic attenuation in two-dimensional packings14 if we select ωG as ω0 in eqn (13) (note that the jamming scaling of the disorder parameter γ varies on the selection of the normalisation frequency ω0).
Overall, our findings highlight that jamming scaling laws play a central role in governing elastic fluctuations and their impact on the acoustic attenuation. Nonetheless, the numerical character of the disorder parameter employed in HET remains poorly characterised; clarifying which fluctuations it captures and their scaling near jamming is necessary before HET can be applied to the attenuation prefactor. To resolve these issues, systematic studies at lower pressures and larger system sizes, direct measurements of spatial correlations of local elastic moduli, and quantitative comparisons with acoustic scattering data will be crucial.77,80–84 Pursuing these directions should clarify how universal the observed scalings are and under which physical conditions the HET-based description becomes predictive.
| N/p | 10−2 | 10−3 | 10−4 | 10−5 | 10−6 | 10−7 | 10−8 |
|---|---|---|---|---|---|---|---|
| Harmonic | |||||||
| 1000 | 11 958 |
11 825 |
11 472 |
10 693 |
10 691 |
— | — |
| 4000 | 10 192 |
10 157 |
10 054 |
9832 | 9820 | — | — |
| 8000 | 5800 | 5796 | 5751 | 5700 | 5700 | — | — |
32 000 |
1530 | 1530 | 1527 | 1513 | 1510 | — | — |
64 000 |
690 | 690 | 688 | 681 | 681 | — | — |
128 000 |
407 | 407 | 407 | 407 | 405 | — | — |
| Hertzian | |||||||
| 2000 | 8047 | 8044 | 8014 | 7943 | 7987 | 7960 | 7935 |
32 000 |
1800 | 1800 | 1799 | 1794 | 1767 | 1742 | — |
| N/p | 2 × 10−2 | 10−2 | 10−3 | 10−4 | 10−5 | 10−6 | 10−7 | 10−8 |
|---|---|---|---|---|---|---|---|---|
| Harmonic | ||||||||
| 1000 | 10 945 |
10 556 |
10 312 |
9628 | 9145 | 9075 | 9126 | — |
| 4000 | 6013 | 6017 | 5981 | 5863 | 5510 | 4718 | 4551 | — |
| 8000 | 3709 | 3708 | 3704 | 3664 | 3724 | 3538 | 3421 | — |
32 000 |
1330 | 1330 | 1330 | 1329 | 1317 | 1298 | 1163 | — |
64 000 |
696 | 696 | 696 | 695 | 694 | 648 | 426 | — |
| Hertzian | ||||||||
| 1000 | 7992 | 7986 | 7946 | 7820 | 7589 | 7135 | 6964 | 5699 |
32 000 |
— | 576 | 576 | 576 | 574 | 575 | 556 | 289 |
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