Electronic pump regulates Fe–Co catalytic center to enhance advanced oxidation performance
Abstract
Constructing efficient electron transport channels in metal–organic frameworks (MOFs) is critical for boosting peroxymonosulfate (PMS) activation. We fabricated a Co-doped MIL-101(Fe)-NH2 catalyst, where Fe–Co orbital coupling constructs an electron pump for directional electron transfer to boost PMS activation and 1O2-mediated antibiotic degradation.

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