Integrated dual-confinement effects of quantum dots and spatial CO2 activation for enhanced photoreduction performance

Abstract

A novel dual-confinement photocatalyst based on Co3S4 quantum dots and NiAl-LDH enables efficient CO2 photoreduction by coupling charge separation with surface activation. An interfacial electric field drives electron accumulation at hydroxyl-rich confined sites, lowers the COOH* formation barrier, and affords a CO evolution rate 17.8-fold higher than that of pristine NiAl-LDH.

Graphical abstract: Integrated dual-confinement effects of quantum dots and spatial CO2 activation for enhanced photoreduction performance

Supplementary files

Article information

Article type
Communication
Submitted
17 Apr 2026
Accepted
27 May 2026
First published
27 May 2026

Chem. Commun., 2026, Advance Article

Integrated dual-confinement effects of quantum dots and spatial CO2 activation for enhanced photoreduction performance

J. Zheng, X. Zhao, Y. Li, Z. Song and Z. Liu, Chem. Commun., 2026, Advance Article , DOI: 10.1039/D6CC02356H

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