Phonon bottleneck limits vortex-induced quasiparticle relaxation in epitaxial NbN thin films

Abstract

We present a comprehensive experimental analysis of vortex-driven quasiparticle dynamics in epitaxial NbN thin films under high magnetic fields. By tracking the Larkin–Ovchinnikov instability velocity as a function of temperature and field, we use the well-known field-independent plateau regime in vortex velocity to extract the quasiparticle relaxation time τ. From this plateau, we extract characteristic recombination times ranging from 80 to 10 ps between 8 K and Tc. Comparing our results with previously reported values for NbN and other superconducting systems, we propose a unified scenario where the superconducting gap and temperature jointly govern the phonon bottleneck limiting recombination. The systematic growth of τ at low temperature, consistent with the expected T3 dependence of phonon-limited heat evacuation through the substrate, suggests a universal trend across different materials and device architectures. These findings provide insights into non-equilibrium superconductivity and establish a fundamental limit for quasiparticle relaxation that constrains the speed of next-generation cryogenic superconducting technologies.

Graphical abstract: Phonon bottleneck limits vortex-induced quasiparticle relaxation in epitaxial NbN thin films

Article information

Article type
Paper
Submitted
27 Jun 2025
Accepted
26 Sep 2025
First published
02 Oct 2025

J. Mater. Chem. C, 2025, Advance Article

Phonon bottleneck limits vortex-induced quasiparticle relaxation in epitaxial NbN thin films

N. Haberkorn, J. C. Zapata, Y. Lee, C. Lee, J. Yun and J. Kim, J. Mater. Chem. C, 2025, Advance Article , DOI: 10.1039/D5TC02466H

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