Unveiling Li+ storage behaviors in two-dimensional organic frameworks through an “adsorption–intercalation–adsorption/filling” mechanism

Lina Zhong; Wenlu Sun; Luting Xie; Lei Fang; Hui Zhang; Huabin Kong; Zhilong Quan; Lifeng Cai; Hongwei Chen

doi:10.1039/D5CC00483G

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Unveiling Li⁺ storage behaviors in two-dimensional organic frameworks through an “adsorption–intercalation–adsorption/filling” mechanism†

Lina Zhong,‡^a Wenlu Sun,‡^a Luting Xie,‡^a Lei Fang,^a Hui Zhang,^c Huabin Kong,

^a Zhilong Quan,*^a Lifeng Cai^b and Hongwei Chen

*^a

Author affiliations

* Corresponding authors

^a College of Materials Science and Engineering, Huaqiao University, Xiamen, Fujian Province, China
E-mail: hwchen@hqu.edu.cn

^b Key Laboratory of Ecological Environment and Information Atlas, Fujian Provincial University, Putian University, Putian, Fujian Province, China

^c National Key Laboratory of High-efficiency Utilization of Coal and Green Chemical Engineering, Ningxia University, Yinchuan, Ningxia 750021, China

Abstract

2D organic frameworks, with microcrystalline layers, show potential as lithium-ion battery anodes. This study explores their ion storage mechanism through the CTF model, revealing an “adsorption–intercalation–adsorption/filling” process.

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Article information

DOI: https://doi.org/10.1039/D5CC00483G
Article type: Communication
Submitted: 25 Jan 2025
Accepted: 12 Mar 2025
First published: 02 Apr 2025

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Chem. Commun., 2025,61, 6336-6339

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Unveiling Li⁺ storage behaviors in two-dimensional organic frameworks through an “adsorption–intercalation–adsorption/filling” mechanism

L. Zhong, W. Sun, L. Xie, L. Fang, H. Zhang, H. Kong, Z. Quan, L. Cai and H. Chen, Chem. Commun., 2025, 61, 6336 DOI: 10.1039/D5CC00483G

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