Issue 98, 2021

Oxidative coupling of methane over Mo–Sn catalysts

Abstract

A novel Mo–Sn catalyst for the oxidative coupling of methane was designed using a hydrothermal method. At 650 °C, the conversion of methane was 8.6% and the selectivity of the C2 hydrocarbons reached as high as 98.1% over the Mo1Sn3 catalyst, with a CO2 selectivity of only 0.8%. We demonstrated that the deep oxidation of methane to CO2 was further inhibited due to the synergistic effects of moderately strong basic sites and reactive oxygen species on the catalyst surface.

Graphical abstract: Oxidative coupling of methane over Mo–Sn catalysts

Supplementary files

Article information

Article type
Communication
Submitted
30 Aug 2021
Accepted
02 Nov 2021
First published
02 Nov 2021

Chem. Commun., 2021,57, 13297-13300

Oxidative coupling of methane over Mo–Sn catalysts

L. Yan, J. Zhang, X. Gao, F. Song, X. Wang, T. Zhang, X. Liu, X. Meng, Q. Zhang, Y. Han and Y. Tan, Chem. Commun., 2021, 57, 13297 DOI: 10.1039/D1CC04821J

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