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The effect of cationic concentration on controlling the interlayer spacings of graphene oxide (GO) membranes is systemically studied. It was found that a higher concentration leads to narrower interlayer spacings, and thus, ions in salt solutions were effectively rejected. This provides a new avenue for ion separation using graphene-based membranes.

Graphical abstract: Effects of cationic concentration on controlling the interlayer spacings for highly effective ion rejection via graphene oxide membranes

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