Wenli
Li
ab,
Yiting
Yu
*ab and
Weizheng
Yuan
*ab
aKey Laboratory of Micro/Nano Systems for Aerospace (Ministry of Education), Northwestern Polytechnical University, Xi'an 710072, China. E-mail: yyt@nwpu.edu.cn
bShaanxi Province Key Laboratory of Micro and Nano Electro-Mechanical Systems, Northwestern Polytechnical University, Xi'an 710072, China. E-mail: yuanwz@nwpu.edu.cn
First published on 11th December 2018
Planar super-oscillatory lenses (SOLs) can exert far-field foci beyond the diffraction limit free from the contribution of evanescent waves. However, the reported design methods of SOLs are always complicated and divergent, leading to a poor control over the desired focusing patterns. Furthermore, the existing device sizes of SOLs are mainly within hundreds of micrometers accompanied by a subwavelength-scale feature size. Here, we propose a general optimization design model for realizing flexible focusing patterns, e.g. multifocal and achromatic contours. Additionally, a novel design called the chromatic-customized SOL fighting against the dispersion rule of traditional diffractive optical elements (DOEs) is also demonstrated based on the proposed flexible algorithm. The diameters for all the SOLs reach 12 mm with 30 μm minimum feature size, which can be easily fabricated by employing the conventional optical lithography technique. Such centimeter-scale, light weight and low-cost lenses reveal new capacities of arbitrarily customized optical patterns in various interdisciplinary fields including parallel particle trapping, full-color high-resolution imaging, and compact spectral imaging.
On the other hand, a non-invasive optical far-field focusing and imaging technique based on super-oscillatory lenses (SOLs) was also proposed.13–16 The optical super-oscillation phenomenon is the delicate interference of far-field propagating waves carrying the fine physical details of objects, and it can be accurately engineered to achieve sub-diffraction-limit foci, even smaller than the size defined as the super-oscillatory criterion 0.38λ/NA (where NA is the numerical aperture).17,18 However, the peak-intensity ratio between the strongest side-lobe and central main-lobe is 16.2% for super-oscillation hotspots, and the focal spot can be further reduced with the exponentially increasing side-lobe intensity.19 Consequently, the small super-oscillation hotspots are always accompanied by the inevitably moderate side lobes, bringing a certain inconvenience for practical applications, especially in the field where it doesn't need a too small hotspot but a wide enough effective field of view for optical imaging. To make a reasonable balance among centimeter-scale lens, the subwavelength hotspot, extremely long working distance and relative weak side lobes for practical applications, we confined the hotspots within the range between the super-oscillatory criterion and the Rayleigh criterion20 to customize the centimeter-scale planar super-resolution lens with an extremely long working distance.
In the previous binary SOL-based super-focusing work, SOLs were optimized by means of the genetic algorithm (GA)13,21 or binary particle swarm optimization (BPSO) algorithm,16,22 for which complicated approaches were required to construct super-oscillatory light fields, however with low-efficiency control. In our previous work, we proposed the multi-objective and multi-constraint optimization method to acquire super-focusing light fields with patterns of optical needle23 or multi-foci.24 However, the demonstrated method needs a large number of initial populations to launch the iterative process and shows a poor convergence. To develop a highly efficient and controllable iterative procedure, we are here aiming to substitute the constraints as penalty functions into GA combined with the vectorial angular spectrum (VAS) theory. Consequently, the existing multi-objective and multi-constraint problem is transformed to an unconstrained multi-objective optimization issue which can easily meet various design requirements, solving the problems of divergence and low efficiency.
Restrictions in the design complexity and bulky form for the traditional diffractive multifocal and achromatic lenses are inevitable.25–28 We handle these two optical patterns that can be arbitrarily achieved through a single SOL. In practice, the far-field super-resolution multifocal lens and achromatic lens can find their various opportunities in parallel particle trapping, three-dimensional data storage and full-color high-resolution imaging. It's worth mentioning that the achromatic design of SOL was made possible through creating different foci of long depths and making them partially overlap to focus at the same point.29 Nevertheless, it could not be treated as a direct way to realize the achromatic optical contour, and a much more controllable design is urgently needed. In addition, the proposed optimization algorithm can be applied to exploit an achromatic-customized optical field which manifests noticeable contradiction to the dispersive rule of traditional diffractive optical elements (DOEs), namely a longer wavelength brings about a shorter focal length. Based on our novel design idea, an achromatic-customized SOL can be realized at will to develop its promising applications in compact diffractive spectral imaging systems and portable spectrometers.
The other key factor that influences the practical applications of planar SOLs is the fabrication process. To make a general survey on the fabrication technologies for the reported SOLs,13,22,30–38 as shown in Fig. 1, most devices were fabricated by focused ion beam (FIB) milling or electron beam lithography (EBL) because of their deep-subwavelength fabrication capability. Owing to the characteristics of high cost, time consumption, and specific material requirements, these two common fabrication methods cannot be the first choice to prepare devices on a large scale. Notably, parallel fabrication of planar SOLs is becoming the main trend. Recently, a SOL with a 1.2 μm line width was first proposed19 instead of the subwavelength-scale feature size. However, the diameter of the reported device fabricated by deep ultra-violet (DUV) lithography was just 600 μm bringing a big difficulty in integrating with the existing centimeter-scale optical systems. More recently, direct laser writing (DLW) lithography was employed to fabricate a 600 μm-diameter SOL,38 in which the whole device was printed through several square regions and an apparent misalignment could be found. To better meet the requirements of low-cost and parallel fabrication for optical elements, we push the smallest line width of our planar SOLs to 30 μm and make their diameters reach 12 mm, which is known to the best of our knowledge as the largest single planar SOL until now. Therefore, planar SOLs with large sizes add the compatibility to the current optical components. On the other hand, the tens of micrometers feature size of the proposed SOLs can be easily fabricated by the normal lithography process at the wafer level.
Such centimeter-scale, light weight and low-cost lenses accompanied by flexible customized optical patterns can develop their wide applications in interdisciplinary fields including parallel particle trapping, full-color high-resolution imaging, and compact spectral imaging systems.
Fig. 2 Schematic illustration of sub-diffraction-limit focusing by SOLs, behaving like common diffractive optical elements (DOEs). |
To provide a general programming model for controllably designing SOLs, we restrain the intensity I along two orthogonal directions, including the optical axis and transverse axes in every focal plane. A specific fluctuation range of the side lobe is set to ensure the light field as required. If the value is improper, it may be difficult to converge to an optimal solution. After evaluating the energy distribution between the side lobe and the central spot, a side lobe factor of 0.3 is chosen in our design. We employ the GA based on the MATLAB programming language to design binary phase-type (0, π) SOLs that implement the predefined axial-intensity modulation over a given region. Hence, a general universal optimization model is built up as in eqn (1) and (2).
Minimize
(1) |
Subject to
(2) |
Here, we assign a weighted coefficient wj to each objective function Ij, so that the problem can be converted to a single-objective problem with the objective function defined as in eqn (3).
(3) |
In our previous iterative processes,23,24 the constrained conditions were directly put into the algorithm to select the optimal solution with a distinct divergence. Indeed, there is always a need for a large number of initial individuals to launch the optimization and the desired results could not be generated at once. To solve the mentioned issue, the constrained conditions are changed as penalty function and put into the iterative process in which the parameters can be tuned according to the specific demands on the SOLs. Obviously, the multi-objective and multi-constraint optimization problem can now be transformed to the unconstrained multi-objective problem, resulting in a highly efficient optimization process. Therefore, the whole algorithm is made more flexible and can be utilized to controllably design SOLs according to specific applications. The entire design procedure is illustrated in Fig. 3. The major steps are as follows: first, to create random masks as initial populations and calculate objective functions for different focal lengths and wavelengths of each mask served as the fitness value; second, to change the given constrains as penalty functions and add to the objective functions; third, to iteratively perform the genetic operations among the population (selection, crossover and mutation) and reinsert the offspring population to the original parental population according to the fitness value of each mask until the termination criterion is satisfied. In the end, the best structural mask in the population is achieved. To realize arbitrarily focusing optical patterns designed for the planar SOLs, the super-resolution multifocal SOL and achromatic SOL are optimized which can find their wide uses in parallel particle trapping and high-resolution label-free microscopy instead of the traditional bulky and complicated DOEs. Furthermore, the achromatic-customized SOL based on the proposed flexible algorithm is firstly demonstrated to expand its new applications in the compact diffractive spectral imaging system. What should be also mentioned here is that the diameters of the designed SOLs are all set as large as 12 mm to enhance their compatibility with the commercialized optical system. Moreover, the 30 μm smallest annular size of the designed SOLs makes it possible to fabricate the centimeter-scale device through the normal lithography process. To verify the calculation efficiency of the proposed algorithm, the GA performance tracking of the designed three SOLs is illustrated in the ESI.† It is noteworthy that the three SOLs can be obtained just through nearly 20 generations regardless of their large dimensions, and a highly efficient and convergent iterative process can be developed.
For clarity, three SOLs with various purposes, i.e. for the multifocal optical field, for the achromatic case and achromatic-customized design, are denoted as sample #1, #2, and #3 in the following discussion, respectively. The detailed design parameters and the corresponding calculated Rayleigh diffraction limit for SOLs #1–#3 are given in the ESI.†
Fig. 5 The device images obtained by both optical and electronic microscopes for the fabricated SOLs. |
The designed centimeter-scale ultrathin multifocal SOL can make its great progress in the miniaturization of optical systems such as imaging systems, detectors, optical data storage, laser printing, optical free-space communications etc.
Minimize
(4) |
Subject to
(5) |
Minimize
(6) |
Subject to
(7) |
To illustrate the proposed optimization model, we design a SOL that could simultaneously focus the three primary colors at the same position, producing intuitively perceived white light. As is well known, these three colors can be mixed to generate a computer display. The computed intensity distributions in the longitudinal cross-section are presented in Fig. 7a. The corresponding experimental data are shown in Fig. 7b. The optical contours in the focal planes for R, G and B wavelengths are screened in Fig. 7e1–e3. The corresponding normalized intensity distributions are also shown in Fig. 7d, which shows an excellent agreement with each other. The detailed computed hotspot sizes reach 0.74λR at λR = 640 nm, 0.81λG at λG = 532 nm and 0.74λB at λB = 405 nm. Besides, the experimental hotspots for the three wavelengths were (0.74 ± 0.02)λR, (0.81 ± 0.01)λG and (0.74 ± 0.02)λB, respectively. Obviously, the computed and measured results are all beyond the Rayleigh diffraction limit. As expected, we could acquire a ‘white’ sub-diffraction hotspot by fusing the images of the three selected RGB wavelengths as seen in Fig. 7e4.
Actually, we didn't consider the material dispersion induced phase modulation difference at other wavelengths (>π for short wavelengths, <π for longer wavelengths) in the optimization process. To verify the robustness of the focusing behaviour on the non-ideal 0/π phase modulation, the optimized phase transmittance has been changed to 0/0.873π and 0/1.5π, and the focusing patterns of the achromatic SOL are shown in the ESI.† We can find out that the two kinds of non-ideal phase modulation seem to function little on the focusing behavior of the achromatic SOL, which shows a relatively good robustness in the dielectric layer. Nonetheless, the suitable phase modulation matching with the corresponding incident wavelength should be taken into consideration in the optimization to obtain a more precise control over the focal contours of the achromatic SOL. Additionally, more than three wavelengths can be designed in the same way based on the proposed algorithm (see the ESI†), and a continuously broadband achromatic SOL can be achieved in the near future.
Minimize
(8) |
Subject to
(9) |
The computed intensity distributions in the longitudinal cross-section are presented in Fig. 8a. The corresponding experimental data are shown in Fig. 8b. The optical contours in the focal planes for R, G and B wavelengths are screened in Fig. 8e1–e3. The corresponding normalized intensity distributions for the simulated and experimental ones in the focal planes are also shown in Fig. 8d, which shows a good agreement with each other. The detailed computed hotspot sizes are 0.77λR at λR = 640 nm, 0.78λG at λG = 532 nm and 0.77λB at λB = 405 nm, respectively. Correspondingly, the experimental hotspots for the three wavelengths are (0.77 ± 0.02)λR, (0.78 ± 0.06)λG and (0.80 ± 0.05)λB, respectively. The computed and measured results are all beyond the Rayleigh diffraction limit except for the one at λB, whose causes are still under investigation, mainly from two aspects, i.e. fabrication imperfections and measurement errors. For the blue wavelength, the detector built in the customized system seems to show a sensitive response to the wavelength and the homemade fiberized coupled laser of 405 nm seems to show a relatively worse stability which may lead to the increasing depth of focus at the wavelength of 405 nm. Additionally, the slight divergence of the incoming light (the fiber collimator only works well for the limited spectral range) may also influence the focusing performance of SOLs. In line with the designs of multifocal and achromatic SOLs, the number of wavelengths concerned is not a limitation on employing the proposed optimization method.
The findings can pave the way for a new model to establish spectral imaging systems and data storage. Besides, the high freedom of controlling the optical components according to the customized requirements can increase the performance and number of functionalities of this kind of light weight planar optical device.
To conduct the low-cost and parallel fabrication of planar optical elements, we put forward a wafer-level fabrication of planar SOLs in which the normal lithography process has been utilized instead of the high cost fabrication ways such as FIB milling and EBL methods. We experimentally demonstrate the far-field focusing properties of the three designed SOLs. Encouragingly, the obtained results agree well with the simulations. The developed SOLs create sub-diffraction hotspots by delicate constructive interference of propagating optical waves and can be tuned intricately to achieve a desired light field. Since less ring belts can lead to a coarse regulation of the light field after the lens surface, an increased number of concentric rings can contribute to the interference of diffracted beams and enlarge the degrees of freedom in optimization design, especially for broadband cases. It's worth noting that most of the light energy of SOLs is contributed to the large side lobes around the central sub-diffraction-limit hotspots, and there needs a tradeoff between the spot size and focusing efficiency. Similar to the binary phase-type Fresnel zone plate (FZP), being famous as diffractive lenses, the maximum efficiency that can be achieved is always limited to around 40% in theory.17,47 As a matter of fact, the low level of throughput efficiency may be prohibitive for some demanding applications but may be tolerable for others. For phase-type SOLs, multiple phase levels instead of the binary phase would be beneficial to reduce the side lobes and increase the focusing efficiency. Besides, the low focusing efficiency of SOL could be still applicable for practical applications in the case of high-energy laser sources and high-sensitivity detectors. Additionally, the proposed design methods can be available for all the wavelengths.
The unprecedented design freedom of planar SOLs will greatly expand the range of applications of micro-optics and integrated optics. We hope that the designed and fabricated centimeter-scale multifocal SOL, achromatic SOL and achromatic-customized SOL can serve as powerful super-resolution focusing and imaging tools for a wide range of applications in parallel data storage, high-resolution broadband noninvasive imaging, low-cost fiberized microscopy, portable Raman spectrometers for super-resolution bio-imaging, optical coherence tomography imaging and micro/nanofabrication.
Footnote |
† Electronic supplementary information (ESI) available: details of performance tracking, design parameters, optical measurement, and super-achromatic SOL design. See DOI: 10.1039/c8nr07985d |
This journal is © The Royal Society of Chemistry 2019 |