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Abstract | Cited by

‘Hangman-type’ PNP pincer ligands and their associated Ru complexes undergo sp2–sp3 C–C bond cleavage and subsequent C–C formation processes to form a new, one carbon unit longer backbone motif. DFT and mechanistic studies suggest a mechanism dependent upon arm pyridine coordination and ligand sterics.

Graphical abstract: Unusual rearrangement of modified PNP ligand based Ru complexes relevant to alcohol dehydrogenation catalysis

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