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Abstract | Cited by

The sterically accessible carbide complex, (Cy3P)Cl3Ru[triple bond, length as m-dash]C–PtCl(py)2, acts as a synthon for terminal and bridging carbide fragments that relocate to pincer and A-frame scaffolds upon ligand addition. This concept, benefitting from coordination sphere selection as the concluding step, confronts traditional synthetic strategies and broadens the scope for carbide complexes.

Graphical abstract: Synthons for carbide complex chemistry

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