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Comparative studies of single molecule force spectroscopy and molecular dynamics simulations indicate that natural cellulose is more hydrophobic than amylose at the single-chain level, implying that the hydrophobicities of these polymeric isomers are regulated by only one parameter in the chains, the linkage between the sugar rings.

Graphical abstract: Hydrophilicities of amylose and natural cellulose are regulated by the linkage between sugar rings

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