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Abstract | Cited by

A new method for the synthesis of diverse N-alkylation compounds was developed via an iron-catalyzed etheric Csp3–O cleavage with the C–N bond formation in the reaction of π-activated ethers with various nitrogen-based nucleophiles. In addition, the mechanism of this reaction was investigated.

Graphical abstract: Iron-catalyzed N-alkylation using π-activated ethers as electrophiles

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