The catalytic ammoxidation of isobutane to methacrylonitrile at 673 K proceeds on a new class of Re mixed-oxide SbRe2O6 with alternate (Re2O6)3− and (SbO)+ layers, where ammonia is prerequisite for the C–H bond scission of isobutane.
Selective ammoxidation of isobutane on a crystalline SbRe2O6 catalyst
H. Liu, T. Shido and Y. Iwasawa, Chem. Commun., 2000, 1881 DOI: 10.1039/B005868H
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