Ajmaline was converted into new Gelsemium alkaloids, 19Z-anhydrovobasinediol [(19Z)-taberpsychine] and N-demethoxyrankinidine, via koumidine along the biomimetic sequence, and the absolute configuration of these alkaloids was determined by these transformations.
M. Kitajima, H. Takayama and S. Sakai, J. Chem. Soc., Perkin Trans. 1, 1991, 1773 DOI: 10.1039/P19910001773
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